 This paper presents a novel method to create bi-directionally-aligned T3C2-TX at Fe 304-CNF aerogel composites using vacuum-assisted impregnation of epoxy resin. The resulting composite exhibits superior electromagnetic interference shielding effectiveness compared to other similar composites. Additionally, it has high thermal stability and mechanical strength, making it ideal for use in a variety of applications such as aerospace and weapon manufacturing. This article was authored by Lei Wang, Zheng Lei Ma, Hua Chiu, and others.