 Highlight self-healing graphene and emzene-based composites can be deployed in wearable sensors, supercapacitors, anti-corrosive coatings, electromagnetic interference shielding, electronic skin, and soft robotics. Self-healing graphene and emzene-based composites have shown improved electrical conductivity, mechanical properties, healing efficacy, and energy conversion efficacy. Self-healing structures can open up considerable new horizons in the future of healthcare, sensors, electronics, robotics, supercapacitors, slash batteries, coatings, and biomedicine. This article was authored by Adafaze Airport, Sepida Amati, Navid Rebe, and others.