 Abstract carbon dots, CDs, can be used in sensing, energy storage, and catalysis due to their excellent optical, electrical, and semi-conducting properties. Attempts to optimize these properties through high-order manipulations have been unsuccessful so far. In this study, CDs were assembled into flexible ribbons using superficial ligands which resulted in excellent stability against UV irradiation and heating. These ribbons showed outstanding performance as active layers in transparent flexible membersters with the devices showing good data storage and retention capabilities as well as fast optoelectronic responses. Additionally, the device was able to function effectively as a neuromorphic computing system with integrated storage and computation capabilities with the response time being less than 5.5 NS. This work lays the foundation for wearable artificial intelligence. This article was authored by Lin AI, Ife Pei, Ziki Song, and others. We are article.tv, links in the description below.