A one-year planning grant was awarded by The Andrew W. Mellon Foundation to study the feasibility of establishing Centers of Excellence (CoEs). This study recognizes CoEs as a means to provide new information services that libraries are increasingly expected to deliver in order to meet the needs of twenty-first century research, teaching, and learning. A team of seven librarians from Association of Research Libraries (ARL) libraries interviewed directors of 19 CoEs and staff from seven funding organizations. The study explored the characteristics of CoEs, what makes them successful, and the challenges commonly faced by centers. Criteria were identified for forming, evaluating, and sustaining a Center of Excellence. This video includes presentation of study findings and preliminary recommendations for following a Centers of Excellence model in developing and delivering information services. The results are intended to be useful to funders who have an interest in funding centers, as well as to institutions interested in forming a center, and staff of existing centers who seek new funding.