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Uploaded by DmitriKilin on Apr 3, 2011
The fluorescence signal shown in the bottom panel is split into the dye (red) and dot (blue) contributions. The inserts present the time-dependent localizations of the exciton of the dot and the dye, with the green circle showing the current moment in time. The movie shows evolution after a short pulse excitation for the time interval from 0 to 10 nanoseconds. For details please see Fig. 3 of the following paper:
Kilin, D. S., K. L. Tsemekhman, O. V. Prezhdo, E. I. Zenkevich, C. von Borczyskowski, (2007). "Ab initio study of exciton transfer dynamics from a core-shell semiconductor quantum dot to a porphyrin-sensitizer." Journal of Photochemistry and Photobiology a-Chemistry 190(2-3): 342-351.
http://linkinghub.elsevier.com/retrieve/pii/S1010603007001049
Tags: fluorescence resonance energy transfer, "stimulated emission" "density matrix" "exciton transfer" "quantum dot" "dye sensitizer" "photodynamic therapy" PDT Foerster "time-dependent quantum theory" "time dependent density matrix" "time evolution" "electronic energy transfer" "von Neuman equation" "reduced density matrix" "dipole-dipole interaction" "scientific video" MATLAB "femtosecond spectroscopy" "Redfield equation" "Liouville superoperator" "electronic structure" "transition density" "Liouville space" theory computation "cadmium selenide" "core-shell" "CdSe" "ZnS"
"CdSeZnS DFT" "Core-shell quantum dot" "Cadmium Selenide" "density functional theory" "Zink sulfide" CdSe
http://www.usd.edu/arts-and-sciences/chemistry/dmitri-kilin.cfm
http://test-www.usd.edu/arts-and-sciences/chemistry/kilin.cfm
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Music: Caprice no. 24 / Paganini
scroff77 4 months ago
What's the music on this one?
lucasfibonacci1 5 months ago in playlist More videos from DmitriKilin